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The self-organization of pi-conjugated organic materials forming highly ordered supramolecular architectures has been extensively investigated in the last two decades in view of optoelectronic applications.Indeed, the control of both the mesoseopic and nanoscale organization within thin semiconducting films is the key issue for the improvement of charge transport properties and achievement of high charge carrier mobilities.These well-ordered materials are currently either self-organized semiconducting polymers or liquid crystals [1].