聚电解质复合物在表面活性剂水溶液中的溶解机理

来源 :高等学校化学学报 | 被引量 : 0次 | 上传用户:oppoyy
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
Polyelectrolyte complex formed from diazoresin(DR) as cationic polyelectrolyte and alkaline hydrolysate of styrenemaleic anhydride copolymer(PSMNa) as anionic polyelectrolyte does not dissolve in water or organic solvents due to its ionic crosslinking structure. It was found that the solubility of this complex was greatly enhanced in aqueous solution of sodium dodecyl sulfate(SDS). The solubility of DRPSMNa complex in 0.1 mol/L and 0.15 mol/L SDS aqueous solution was determined to be 0.024 g/mL and 0.033 g/mL respectively. It was also confirmed that the complex from DR and SDS, which does not dissolve in water, can also dissolve in SDS aqueous solution. The decomposition temperature(T d ) of diazonium groups for different complexes was determined by DSC and shows that the T d of DRPSMNa after dissolution in SDS aqueous solution changes to 146 ℃ from the original value of 133 ℃. It was proposed that during the dissolution of PEC in surfactant aqueous solution, the complex is separated to its two components via the interaction between PEC and surfactant molecules at first, then the components dissolve in water. Polyelectrolyte complex formed from diazoresin (DR) as cationic polyelectrolyte and alkaline hydrolysate of styrenemaleic anhydride copolymer (PSMNa) as anionic polyelectrolyte does not dissolve in water or organic solvents due to its ionic crosslinking structure. It was found that the solubility of this complex was greatly The solubility of DRPSMNa complex in 0.1 mol / L and 0.15 mol / L SDS aqueous solution was determined to be 0.024 g / mL and 0.033 g / mL respectively. It was also confirmed that aqueous solution of sodium dodecyl sulfate (SDS) the complex from DR and SDS, which does not dissolve in water, can also dissolve in SDS aqueous solution. The decomposition temperature (T d) of diazonium groups for different complexes was determined by DSC and shows that the T d of DRPSMNa after dissolution in It was proposed that during the dissolution of PEC in surfactant aqueous solution, the complex is sepa rated to its two components via the interaction between PEC and surfactant molecules at first, then the components dissolve in water.
其他文献
本文用实验方法研究了浓度为1500 wppm 的聚丙烯酰胺(PAM)溶液在周期性渐扩渐缩通道内层流流动与换热问题.研究表明,大约经过8个周期后流动进入充分发展阶段,而换热则要经过
对用于F T合成制液态烃的Co/Al2 O3 催化剂进行了程序升温还原研究 ,确定了合适的还原活化温度 (约6 0 0~ 80 0K) ,同时考察了钴负载量和焙烧温度对催化剂活性的影响 .结果表
Au/PATP/PANI (polyaniline) film electrode was prepared by voltamometry in 0.5 mol/L aniline/0.5 mol/L HClO 4 from -0.2—0.8 V at 100 mV/s after selfassembling
:研究了一种用彩色条纹对光栅进行编码的光栅投影三维轮廓术。其中投影光栅用白、红、绿和蓝 4种颜色按照二进制原理对光栅进行编码。用白色条纹和绿色条纹分别代表两位二进
在局部热动平衡条件下,用STA(超组态跃迁阵)模型探索研究和计算Au等离子体在一定温度和密度下的跃迁阵的参数,并用来计算冲击压缩下等离子体的辐射不透明度.
采用浸渍法、机械混合法和水热法制备了Mo/HZSM 5分子筛催化剂 ,考察了Mo含量和在线反应时间对丙烷芳构化反应的影响 ,并以IR ,XRD ,NH3 TPD和XPS等表征手段研究了Mo物种对H
机械损伤是否产生取决于损伤驱动力及损伤抗力,对于陶瓷涂层而言,区别于单质固体的是,其损伤驱动力及损伤抗力二者都与材料本身相关,二者都受涂层与基体材料间的热学及力学匹
本文主要介绍了 3种大分子自组装体系 :含硫化合物在重金属表面的自组装功能膜、聚合物在溶液状态下的自组装体系和聚合物基材上的自组装功能膜。文中还介绍了表征自组装体系
基于从两体关联动力学获得的与扩展时间相关的HartreeFock(ETDHF)方程,研究了核流体动力学模型的理论基础.同时,通过在Wigner表示中定义流矢量和运动应力张量,获得了闭合的核
基于小波变换可以对影像进行正交分解 ,而不丢失原来信号所包含的信息。提出了一种Wallis变换、小波变换和IHS变换相结合用于融合的方法 ,该方法可以有效地提高多光谱影像的空间分辨率 ,同时保持原来多光谱影像的色调。