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本研究制备了一系列不同Nd含量的V2O5-MoO3-Nd2O3/TiO2平板式脱硝催化剂.采用XRD、N2-吸附脱附、XPS、H2-TPR、拉曼光谱、NH3-TPD和红外光谱等表征手段对催化剂进行分析.结果表明:适量的Nd2O3(0.25%、0.5%,质量分数)可以增强V2O5-MoO3/TiO2催化剂的还原性能,增加了催化剂的Oα/(Oα+Oβ)比率,从而提升了催化剂的脱硝活性.然而,过量Nd2O3(0.75%、1%)的添加,会导致催化剂酸性性能的显著降低,造成催化剂脱硝性能的下降.此外,过量Nd的添加还会对催化剂的耐磨性能有负面影响.各催化剂中,VMoNd(0.5%)/Ti催化剂显示了最佳的脱硝活性.并且,该催化剂还显示了优良的抗SO2、H2O性能.“,”A series of plate-type V2O6-MoO3-Nd2O3/TiO2 catalysts with different amounts of neodymium were prepared to investigate the effect of neodymium addition on selective catalytic reduction(SCR)of NO with NH3.XRD,N2-adsorption,XPS,H2-TPR,Raman,NH3-TPD,and FT-IR were used to characterize the catalysts.It is found that with suitable addition of Nd(0.25wt%and 0.5wt%Nd2O3)to V2O5-MoO3/TiO2 catalyst not only improves the reduction property,but also increases the Oa/(Oα+Oβ)ratio of the catalyst,which results in the enhancement of catalytic effiiciency.However,when the content of Nd2O3 is excessive(0.75wt%and 1wt%),the acid sites of the catalysts decrease.Accordingly,the catalytic performance of these catalysts is relatively low.Moreover,the mechanical property of the catalyst declines when the content ofNd2O3 is excessive.Among the catalysts investigated,VMoNd(0.5)/Ti catalyst has the best catalytic performance,and also exhibits good SO2 and H2O resistance.