【摘 要】
：
Three-dimensional (3D) hybrid of nanocarbons is a very promising way to the high-performance design of electrocatalysis materials.However,sp3-like defect struct
【机 构】
：
State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, and School of Ma
论文部分内容阅读
Three-dimensional (3D) hybrid of nanocarbons is a very promising way to the high-performance design of electrocatalysis materials.However,sp3-like defect structure,a combination of high strength and conduction of graphene and carbon nanotubes (CNTs) is rarely reported.Herein,3D neural-like hybrids of graphene (from reduced graphene oxide) and carbon nanotubes (CNTs) have been integrated via sp3-like defect structure by a hydrothermal approach.The sp3-like defect structure endows 3D nanocarbon hybrids with an enhanced carrier transfer,high structural stability,and electrocatalytic durability.The neural-like structure is shown to demonstrate a cascade effect of charges and significant performances regarding bio-electrocatalysis and lithium-sulfur energy storage.The concept and mechanism of “sp3-like defect structure” are proposed at an atomic/nanoscale to clarify the generation of rational structure as well as the cascade electron transfer.
其他文献
Developing low-priced,yet effective and robust catalysts for the nitrogen reduction reaction(NRR) is of vital importance for scalable and renewable electrochemical NH3 synthesis.Herein,we provide the first demonstration of MoS_3 as an efficient and durabl
The hydrogen evolution reaction(HER)via water electrolysis has gained immense research attention.Seawater electrolysis provides great opportunities for sustaina
Lithium-sulfur (Li-S) batteries hold great promises to serve as next-generation energy storage devices because of their high theoretical energy density and envi
Nanostructured scaffolds offer promising opportunities in enabling dendrite-free long-cycle life Li metal anode.The rational design and controllable synthesis of scaffolding architectures are imperative for development of rechargeable Li metal batteries.I
Fast charging and high-power delivering batteries are highly demanded in mobile electronics,electric vehicles and grid energy storage,but there are full of chal
With the rapid exhaustion of fossil energy, the demand for clean and renewable energy is urgently growing. Thermoelectric(TE) materials, which can directly convert waste heat into electrical energy, are attracting great attention to address the energy cri
With the development of stable alkali metal anodes,V2O5 is gaining traction as a cathode material due to its high theoretical capacity and the ability to interc
A composite In-Pb:carbon was successfully synthetized by a two-step mechanochemical synthesis in order to obtain an adequate particles size and structure to inv
A controllable crystallization is of practical importance to produce high-quality perovskite thin films with reduced structural defects.Lewis bases as electron-
Lithium-sulfur(Li-S)batteries possess overwhelming energy density of 2654 Wh kg-1,and are consid-ered as the next-generation battery technology for energy deman