Synthesis and Crystal Structure of a New Zn(Ⅱ) Complex Exhibiting Strong Luminescence

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The title complex,[Zn(ip)2(H2O)2][ZnCl4]·H2O·2DMF 1(ip=imidazo[4,5-f][1,10] phenanthroline),has been synthesized via the slow evaporation of concentrated reaction solution at room temperature.It was characterized by single-crystal X-ray diffraction.Crystal data for C32H36Cl4N10O5Zn2:white prism,0.17mm×0.15mm×0.10mm,monoclinic,space group P2/c,a=11.928(8),b=9.868(6),c=16.520(11),β=104.879(12)°,V=1879(2)3,Z=2,Mr=913.25,Dc=1.614 g/cm3,F(000)=932,μ=1.616 mm-1,λ(MoKα)=0.71073,GOOF=1.045,R=0.0710 and wR=0.1755 for 3055 observed reflections with Ⅰ>2σ(Ⅰ).X-ray diffraction study reveals that the title complex has an interesting 3D architecture via hydrogen bonding interactions and π-π interactions.The IR,TGA,XRD and luminescent properties of complex 1 were also studied. The title complex, [Zn (ip) 2 (H2O) 2] [ZnCl4] .H2O.2DMF1 (ip = imidazo [4,5-f] [1,10] phenanthroline), has been synthesized via the slow evaporation of concentrated reaction solution at room temperature. It was characterized by single-crystal X-ray diffraction. Crystal data for C32H36Cl4N10O5Zn2: white prism, 0.17 mm × 0.15 mm × 0.10 mm, monoclinic, space group P2 / c, a = 11.928 , b = 9.868 (6), c = 16.520 (11) β, β = 104.879 (12) °, V = 1879 (2) 3, Z = 2, Mr = 913.25, Dc = 1.614 g / cm3, F X-ray diffraction analysis shows that (a) = 932, μ = 1.616 mm-1, λ (MoKα) = 0.71073, GOOF = 1.045, R = 0.0710 and wR = 0.1755 for 3055 the title complex has an interesting 3D architecture via hydrogen bonding interactions and π-π interactions. IR, TGA, XRD and luminescent properties of complex 1 were also studied.
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