Palladium-Catalyzed Stereoselective C-Glycosylation of Glycals with Sodium Arylsulfinates

来源 :首届糖合成化学青年高峰论坛会议 | 被引量 : 0次 | 上传用户:lightning11111
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
  An efficient glycosylation method to synthesize 2‐deoxy‐C‐aryl glycosides was developed.This C‐glycosylation strategy is based on a palladium‐catalyzed desulfitative Ferrier‐type coupling reaction of glycals and sodium arylsulfinates.A series of C‐aryl glycosides were obtained in moderate to good yields(41‐74%)with exclusive regio‐ and stereoselectivities.The anomeric selectivity was found to depend on the configuration of the C3 substituent of the glycals.These 2‐deoxy‐C‐aryl glycosides could be readily functionalized by epoxidation or hydroxylation to synthesize many natural C‐aryl glucosides or other important pyran structures.
其他文献
  Iminosugars or azasugars,which exhibit effective inhibition against carbohydrate‐ processing enzymes,have attracted great interest for their potential clin
会议
Antitumor vaccines,which aim to boost patients own immune system to cleartumor cells,are very promising for cancer immunotherapy.Tumor‐associated membrane glyc
会议
  Scientific research on proteins has been a hot area in the discipline of life science,as it is an essential means for people to explore and understand life.
会议
Many peptide‐based therapeutics have short circulatory half‐lives.We report here that the pharmacokinetics of an anti‐HIV peptide drug(T20) can be dramatical
会议
Novel synthesis of various sugar alkynones and dialkynones has been achieved by palladium catalyzed coupling reactions of diverse sugar alkynes with substituted
会议
  以海洋半乳聚糖琼胶(AA)、κ‐卡拉胶(KCA)和ι‐卡拉胶(ICA)为原料,采用多聚磷酸‐三正丁胺体系对3 种海洋半乳聚糖进行磷酸化修饰,并通过磷酸基团含量及取代度测定、红
  A novel noncovalent strategy to constructchemically synthesized glycopeptidevaccines has been designed toinduce a robust immune response and to dramatically
会议
  脑膜炎奈瑟菌每年可引起上百万例脑膜炎和败血症,发展一种基于脂多糖核心结构的新型疫苗将可以预防脑膜炎和败血症.脑膜炎奈瑟菌中共存的脂多糖核心四糖由于含有高碳糖He
会议
OAADPR(O‐Acetyl‐ADP‐Ribose) is a metabolite product of nicotinamide adenine dinucleotide(NAD+)‐dependent enzymes,histone deacetylases,named as Sirtuins as w
会议
Lipochitooligosaccharide Nod factors play a key role in the initiation of the symbiotic associations between legume plants and nitrogen-fixing bacteria.However,
会议