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According the multilayer study of CO2 system including DIC,Alk,pH and pCO2 and carbon fluxes in Yellow Sea,South China Sea and Qingdao Coastal,the results are as following: 1.The surface seawater was divided into three layers: surface microlayer (SML),subsurface layer (SSL) and surface layer (SL).Multilayer study of CO2 system including dissolved inorganic carbon (DIC),alkalinity (Alk),pH and partial pressure of CO2 (pCO2) was carried out in China SOLAS plan.The vertical distribution,horizontal distribution and temporal distribution (annual-variation,seasonal-variation,diurnal variation) of marine-geography-chemistry are studied.In aspect of vertical-distribution,it is the first time to study the vertical-microstructure of surface seawater in turn of SML→SSL→SL…….There are 48 figures on multilayer-horizontal distribution,and 24 figures on multilayer-temporal distribution.Meanwhile,the relativity of DIC,Alk,pH,pCO2 versus temperature/salinity/longitude/latitude and the relativity of calculated value versus experimental value agree with the internal-international reports well.