Epitaxial growth and transport properties of compressively-strained Ba2IrO4 films

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Ba2IrO4 is a sister compound of the widely investigated Sr2IrO4 and has no IrO6 octahedral rotation nor net canted antiferromagnetic moment,thus it acts as a system more similar to the high-Tc cuprate.In this work,we synthesize the Ba2IrO4 epitaxial films by reactive molecular beam epitaxy and study their crystalline structure and transport properties under biaxial compressive strain.High resolution scanning transmission electron microscopy and x-ray diffraction confirm the high quality of films with partial strain relaxation.Under compressive epitaxial strain,the Ba2IrO4 exhibits the strain-driven enhancement of the conductivity,consistent with the band gap narrowing and the stronger hybridization of Ir-t2g and O-2p orbitals predicted in the first-principles calculations.
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