Facile construction of honeycomb-shaped porous carbon electrode materials using recyclable sodium ch

来源 :中国科学:技术科学(英文版) | 被引量 : 0次 | 上传用户:xdlclub
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Carbon materials are the preferred anode materials for Li-ion batteries.Here,we propose an easy and sustainable strategy to prepare honeycomb-shaped porous carbon (HPC) electrode materials through a process involving simple calcination and subsequent water washing by using polyvinyl-pyrrolidone (PVP) as carbon source and NaC1 as pore-forming agent.A controllable cavity size and distribution of the carbon materials can be readily obtained solely by adjusting the NaCl amount.Results showed that the optimized HPC sample had a relatively uniform cavity distribution and a highly porous structure.Moreover,the special honeycomb-shaped structure was conducive to the electronic conductivity of the electrode materials,provided a short path for Li-ion transport and a wide interface with the electrolyte,and buffered the volume change of active materials.The special honeycomb-shaped structure was also maintained well after long cycles,which improved electrode stability.When used as anode materials for Li-ion batteries (LIBs),the sample demonstrated excellent cycling stability and rate performance,with a high specific capacity of 230 mA h g 1 and a reversible capacity of 197 mA h g-1,after 1200 cycles at 2 C.Overall,we introduced a simple strategy for the potential mass production of porous carbon materials for LIBs.
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