Molecular and Crystal Structure of 1-(4-Chlorophenyl)-3-(4-Nitrophenyl)-1-Triazene

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The title compound,1|(4|Chlorophenyl)|3|(4|Nitrophenyl)|1|Triazene, crystallized in the orthorhombic system, space group Pbca, with a=13.793(2), b=10.843(2), c=16.851(2), V=2520.2(7) 3 D c =1.458g/cm 3, Z =8, C 12 H 9ClN 4O 2, M r=276.68, μ (Mo Kα )=0.306mm -1 , F (000)=1136. The structure was refined to R=0.0372, wR =0.0786 for 1216 reflections ( I>2σ(I )). The title molecule has trans geometry about the central triazenyl linkage. The dihedral angle between the two phenyl rings is only 5.8(2)°. They are also nearly coplanar with the triazenyl. The screw related molecules are connected by hydrogen bond N(3)-H…O(2) and form the zigzag chains. The polar molecular chains are antiparallelly stacked through π…π interactions. The interstack interaction is mainly van der Waals force. The title compound, 1 | (4 | Chlorophenyl) | 3 | (4 | Nitrophenyl) | 1 | Triazene, crystallized in the orthorhombic system, space group Pbca, with a = 13.793 (2) b = 10.843 (2) c = 16.851 (2)  V = 2520.2 7 3 D c = 1.458 g / cm 3 Z = 8 C 12 H 9 ClN 4 O 2, M r = 276.68, μ (Mo Kα) = 0.306 mm -1, F (000) = 1136. The structure was refined to R = 0.0372, wR = 0.0786 for 1216 reflections (I> 2σ The geometry of the central triazenyl linkage. The dihedral angle between the two phenyl rings is only 5.8 (2) °. They are also nearly coplanar with the triazenyl. The screw related molecules are connected by hydrogen bond N (3) -H ... O (2) and form the zigzag chains. The polar molecular chains are antiparallelly stacked through π ... π interactions. The interstack interaction is mainly van der Waals force.
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