【摘 要】
：
Conventional oven drying (COD) and supercritical drying (SCD) methods were applied to the preparation of Mn-substituted hexaaluminate (BaMnAl11O19-α) catalysts
【机 构】
：
Laboratory of Natural Gas Utilization and Applied Catalysis, Dalian Institute of Chemical Physics,Ch
论文部分内容阅读
Conventional oven drying (COD) and supercritical drying (SCD) methods were applied to the preparation of Mn-substituted hexaaluminate (BaMnAl11O19-α) catalysts. The effect of drying methods on phase composition, specific surface area, pore structure, reduction behavior of Mn3+ ions, and combustion activity of the samples was investigated. The homogenous mixing of the components in the sol-gel process could be maintained by SCD, and the hexaaluminate phase was almost the only phase of the resulting materials after calcination. H2-TPR revealed that the Mn3+ ions in the sample obtained by SCD were easier to be reduced than that by COD. Moreover, the samples obtained by SCD have higher surface area, narrower pore size distribution, and higher combustion activity than those obtained by COD.
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