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THE metastable CO(a~3Ⅱ) molecule is known to be an important energy carrier. Its energytransfer reactions have been greatly interesting the dynamics workers. Previous studies of theenergy transfer reactions between CO(a~3Ⅱ) and NO(X~3Ⅱ_i) were mainly made in flow sys-tems. The state-to-state process in the energy transfer between them were seldomstudied. Yu et al. investigated the reaction of CO(a~3Ⅱ) with NO(X~3Ⅱ_i) under the condi-