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The Magnetoelectric (ME) composites with composition (y) Ni0.85Cd0.1Cu0.05Fe2O4 + (1-y) BaTiO3,(0.0 < y < 1.0) were synthesized by conventional solid state reaction method.The presence of constituent phases was confirmed by X-ray diffraction studies.Scanning electron microscopy was used to study the surface morphology of the composites.